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2020


Transient coarsening and the motility of optically heated Janus colloids in a binary liquid mixture
Transient coarsening and the motility of optically heated Janus colloids in a binary liquid mixture

Gomez-Solano, J., Roy, S., Araki, T., Dietrich, S., Maciolek, A.

Soft Matter, 16, pages: 8359-8371, Royal Society of Chemistry, August 2020 (article)

Abstract
A gold-capped Janus particle suspended in a near-critical binary liquid mixture can self-propel under illumination. We have immobilized such a particle in a narrow channel and carried out a combined experimental and theoretical study of the non-equilibrium dynamics of a binary solvent around it – lasting from the very moment of switching illumination on until the steady state is reached. In the theoretical study we use both a purely diffusive and a hydrodynamic model, which we solve numerically. Our results demonstrate a remarkable complexity of the time evolution of the concentration field around the colloid. This evolution is governed by the combined effects of the temperature gradient and the wettability, and crucially depends on whether the colloid is free to move or is trapped. For the trapped colloid, all approaches indicate that the early time dynamics is purely diffusive and characterized by composition layers travelling with constant speed from the surface of the colloid into the bulk of the solvent. Subsequently, hydrodynamic effects set in. Anomalously large nonequilibrium fluctuations, which result from the temperature gradient and the vicinity of the critical point of the binary liquid mixture, give rise to strong concentration fluctuations in the solvent and to permanently changing coarsening patterns not observed for a mobile particle. The early time dynamics around initially still Janus colloids produces a force which is able to set the Janus colloid into motion. The propulsion due to this transient dynamics is in the direction opposite to that observed after the steady state is attained.

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link (url) DOI [BibTex]

2020


link (url) DOI [BibTex]


Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles
Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles

Singh, D., Domínguez, A., Choudhury, U., Kottapalli, S., Popescu, M., Dietrich, S., Fischer, P.

Nature Communications, 11(2210), May 2020 (article)

Abstract
Symmetry breaking and the emergence of self-organized patterns is the hallmark of com- plexity. Here, we demonstrate that a sessile drop, containing titania powder particles with negligible self-propulsion, exhibits a transition to collective motion leading to self-organized flow patterns. This phenomenology emerges through a novel mechanism involving the interplay between the chemical activity of the photocatalytic particles, which induces Mar- angoni stresses at the liquid–liquid interface, and the geometrical confinement provided by the drop. The response of the interface to the chemical activity of the particles is the source of a significantly amplified hydrodynamic flow within the drop, which moves the particles. Furthermore, in ensembles of such active drops long-ranged ordering of the flow patterns within the drops is observed. We show that the ordering is dictated by a chemical com- munication between drops, i.e., an alignment of the flow patterns is induced by the gradients of the chemicals emanating from the active particles, rather than by hydrodynamic interactions.

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link (url) DOI [BibTex]


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Axisymmetric spheroidal squirmers and self-diffusiophoretic particles

Pöhnl, R., Popescu, M. N., Uspal, W. E.

Journal of Physics: Condensed Matter, 32(16), IOP Publishing, Bristol, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Tracer diffusion on a crowded random Manhattan lattice

Mej\’\ia-Monasterio, C., Nechaev, S., Oshanin, G., Vasilyev, O.

New Journal of Physics, 22(3), IOP Publishing, Bristol, 2020 (article)

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Wetting transitions on soft substrates

Napiorkowski, M., Schimmele, L., Dietrich, S.

{EPL}, 129(1), EDP Science, Les-Ulis, 2020 (article)

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Blessing and Curse: How a Supercapacitor Large Capacitance Causes its Slow Charging

Lian, C., Janssen, M., Liu, H., van Roij, R.

Physical Review Letters, 124(7), American Physical Society, Woodbury, N.Y., 2020 (article)

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Interplay of quenching temperature and drift in Brownian dynamics

Khalilian, H., Nejad, M. R., Moghaddam, A. G., Rohwer, C. M.

EPL, 128(6), EDP Science, Les-Ulis, 2020 (article)

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Fractal-seaweeds type functionalization of graphene

Amsharov, K., Sharapa, D. I., Vasilyev, O. A., Martin, O., Hauke, F., Görling, A., Soni, H., Hirsch, A.

Carbon, 158, pages: 435-448, Elsevier, Amsterdam, 2020 (article)

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Effective pair interaction of patchy particles in critical fluids

Farahmand Bafi, N., Nowakowski, P., Dietrich, S.

The Journal of Chemical Physics, 152(11), American Institute of Physics, Woodbury, N.Y., 2020 (article)

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Cassie-Wenzel transition of a binary liquid mixture on a nanosculptured surface

Singh, S. L., Schimmele, L., Dietrich, S.

Physical Review E, 101(5), American Physical Society, Melville, NY, 2020 (article)

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Adopting the Boundary Homogenization Approximation from Chemical Kinetics to Motile Chemically Active Particles

Popescu, M. N., Uspal, W. E.

In Chemical Kinetics, pages: 517-540, World Scientific, New Jersey, NJ, 2020 (incollection)

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Energy storage in steady states under cyclic local energy input

Zhang, Y., Holyst, R., Maciolek, A.

Physical Review E, 101(1), American Physical Society, Melville, NY, 2020 (article)

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Numerical simulations of self-diffusiophoretic colloids at fluid interfaces

Peter, T., Malgaretti, P., Rivas, N., Scagliarini, A., Harting, J., Dietrich, S.

Soft Matter, 16(14):3536-3547, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

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2017


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Chemically active colloids near osmotic-responsive walls with surface-chemistry gradients

Popescu, M. N., Uspal, W. E., Dietrich, S.

Journal of Physics: Condensed Matter, 29, IOP Publishing, Bristol, 2017 (article)

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Active colloids in the context of chemical kinetics

Oshanin, G., Popescu, M. N., Dietrich, S.

Journal of Physics A, 50, IOP Pub., Bristol, 2017 (article)

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Microbots Decorated with Silver Nanoparticles Kill Bacteria in Aqueous Media

Vilela, D., Stanton, M. M., Parmar, J., Sánchez, S.

ACS Applied Materials and Interfaces, 9(27):22093-22100, American Chemical Society, Washington, DC, 2017 (article)

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Measurement of second-order response without perturbation

Helden, L., Basu, U., Krüger, M., Bechinger, C.

EPL, 116(6), IOP Publishing, Bristol, 2017 (article)

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Swimming with a cage: low-Reynolds-number locomotion inside a droplet

Reigh, S., Zhu, L. L., Gallaire, F., Lauga, E.

Soft Matter, 13(17):3161-3173, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

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Active Particle Accumulation at Boundaries: A Strategy to Measure Contact Angles

Simmchen, J., Malgaretti, P.

ChemNanoMat, 3(11):790-793, Wiley, Weinheim, 2017 (article)

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Two-fluid model for locomotion under self-confinement

Reigh, S., Lauga, E.

Physical Review Fluids, 2(9), American Physical Society, 2017 (article)

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Bubble gating in biological ion channels: A density functional theory study

Gu\ssmann, Florian, Roth, R.

Physical Review E, 95(6), American Physical Society, Melville, NY, 2017 (article)

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Nematic films at chemically structured surfaces

Silvestre, N. M., Telo da Gama, M. M., Tasinkevych, M.

Journal of Physics: Condensed Matter, 29(7), IOP Publishing, Bristol, 2017 (article)

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Nonadditive interactions and phase transitions in strongly confined colloidal systems

Vasilyev, O., Dietrich, S., Kondrat, S.

Soft Matter, 14(4):586-596, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

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Platinum-free cobalt ferrite based micromotors for antibiotic removal

Parmar, J., Villa, K., Vilela, D., Sánchez, S.

Applied Materials Today, 9, pages: 605-611, Elsevier, Amsterdam, 2017 (article)

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Stationary and time-dependent heat transfer in paradigmatic many-body geometries

Asheichyk, Kiryl

Universität Stuttgart, Stuttgart, 2017 (mastersthesis)

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Perils of ad hoc approximations for the activity function of chemically powered colloids

Popescu, M. N., Uspal, W. E., Tasinkevych, M., Dietrich, S.

The European Physical Journal E, 40, EDP Sciences; Società Italiana di Fisica; Springer, Les Ulis; Bologna; Heidelberg, 2017 (article)

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Transient Casimir Forces from Quenches in Thermal and Active Matter

Rohwer, C. M., Kardar, M., Krüger, M.

Physical Review Letters, 118(1), American Physical Society, Woodbury, N.Y., 2017 (article)

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Rotational motion of dimers of Janus particles

Majee, A.

European Physical Journal E, 40(3), Springer, Berlin, 2017 (article)

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Designing Micro- and Nanoswimmers for Specific Applications

Katuri, J., Ma, X., Stanton, M. M., Sanchez, S.

Accounts of Chemical Research, 50(1):2-11, American Chemical Society, Easton, Pa., 2017 (article)

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Wedge wetting by electrolyte solutions

Mußotter, M., Bier, M.

Physical Review E, 96(3), American Physical Society, Melville, NY, 2017 (article)

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Effect of boundaries on vacuum field fluctuations and radiation-mediated interactions between atoms

Armata, F., Butera, S., Fiscelli, G., Incardone, R., Notararigo, V., Palacino, R., Passante, R., Rizzuto, L., Spagnolo, S.

Journal of Physics: Conference Series, 880, IOP Publishing, Bristol, 2017 (article)

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Non-equilibrium forces after temperature quenches in ideal fluids with conserved density

Hölzl, Christian

Universität Stuttgart, Stuttgart, 2017 (mastersthesis)

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Numerical studies of active colloids at fluid interfaces

Peter, Toni

Universität Stuttgart, Stuttgart, 2017 (mastersthesis)

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[BibTex]


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Smectic phases in ionic liquid crystals

Bartsch, H., Bier, M., Dietrich, S.

Journal of Physics: Condensed Matter, 29(46), IOP Publishing, Bristol, 2017 (article)

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DOI [BibTex]


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Pushing Bacterial Biohybrids to In Vivo Applications

Stanton, M. M., Sánchez, S.

Trends in Biotechnology, 35(10):910-913, Elsevier Current Trends, Amsterdam, Netherlands, 2017 (article)

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Particles with nonlinear electric response: Suppressing van der Waals forces by an external field

Soo, H., Dean, D. S., Krüger, M.

Physical Review E, 95(1), American Physical Society, Melville, NY, 2017 (article)

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Electrolyte solutions at curved electrodes. I. Mesoscopic approach

Reindl, A., Bier, M., Dietrich, S.

The Journal of Chemical Physics, 146(15), American Institute of Physics, Woodbury, N.Y., 2017 (article)

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Self-propelling micro-nanorobots: challenges and fututre perspectives in nanomedicine

Ma, X., Sánchez, S.

Nanomedicine, 12(12):1363-1367, Future Medicine Ltd, London, UK, 2017 (article)

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Salt-induced microheterogeneities in binary liquid mixtures

Bier, M., Mars, J., Li, H., Mezger, M.

Physical Review E, 96(2), American Physical Society, Melville, NY, 2017 (article)

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Forward-backward multiplicity correlations in proton-proton collisions from several GeV to LHC energies

Bravina, L., Bleibel, J., Emaus, R., Zabrodin, E.

EPJ Web of Conferences, 164, EDP Sciences, Les Ulis, 2017 (article)

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Key-lock colloids in a nematic liquid crystal

Silvestre, N. M., Tasinkevych, M.

Physical Review E, 95(1), American Physical Society, Melville, NY, 2017 (article)

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Collective dynamics of laterally confined active particles near fluid-fluid interfaces

Kistner, Irina

Universität Stuttgart, Stuttgart, 2017 (mastersthesis)

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[BibTex]


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Fluctuation induced forces in critical films with disorder at their surfaces

Maciolek, A., Vasilyev, O., Dotsenko, V., Dietrich, S.

Journal of Statistical Mechanics: Theory and Experiment, Institute of Physics Publishing, Bristol, England, 2017 (article)

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Action at a distance in classical uniaxial ferromagnetic arrays

Abraham, D. B., Maciolek, A., Squarcini, A., Vasilyev, O.

Physical Review E, 96(4), American Physical Society, Melville, NY, 2017 (article)

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Cooperative behavior of biased probes in crowded interacting systems

Vasilyev, O., Bénichou, O., Mej\’\ia-Monasterio, C., Weeks, E. R., Oshanin, G.

Soft Matter, 13(41):7617-7624, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

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Nonequilibrium Fluctuational Quantum Electrodynamics: Heat Radiation, Heat Transfer, and Force

Bimonte, G., Emig, T., Kardar, M., Krüger, M.

Annual Review of Condensed Matter Physics, 8, pages: 119-143, 2017 (article)

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A Gaussian theory for fluctuations in simple liquids

Krüger, M., Dean, D. S.

The Journal of Chemical Physics, 146(13), American Institute of Physics, Woodbury, N.Y., 2017 (article)

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Critical Casimir interactions between colloids around the critical point of binary solvents

Stuij, S. G., Labbe-Laurent, M., Kodger, T. E., Maciolek, A., Schall, P.

Soft Matter, 13(31):5233-5249, Royal Society of Chemistry, Cambridge, UK, 2017 (article)

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