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2020


Transient coarsening and the motility of optically heated Janus colloids in a binary liquid mixture
Transient coarsening and the motility of optically heated Janus colloids in a binary liquid mixture

Gomez-Solano, J., Roy, S., Araki, T., Dietrich, S., Maciolek, A.

Soft Matter, 16, pages: 8359-8371, Royal Society of Chemistry, August 2020 (article)

Abstract
A gold-capped Janus particle suspended in a near-critical binary liquid mixture can self-propel under illumination. We have immobilized such a particle in a narrow channel and carried out a combined experimental and theoretical study of the non-equilibrium dynamics of a binary solvent around it – lasting from the very moment of switching illumination on until the steady state is reached. In the theoretical study we use both a purely diffusive and a hydrodynamic model, which we solve numerically. Our results demonstrate a remarkable complexity of the time evolution of the concentration field around the colloid. This evolution is governed by the combined effects of the temperature gradient and the wettability, and crucially depends on whether the colloid is free to move or is trapped. For the trapped colloid, all approaches indicate that the early time dynamics is purely diffusive and characterized by composition layers travelling with constant speed from the surface of the colloid into the bulk of the solvent. Subsequently, hydrodynamic effects set in. Anomalously large nonequilibrium fluctuations, which result from the temperature gradient and the vicinity of the critical point of the binary liquid mixture, give rise to strong concentration fluctuations in the solvent and to permanently changing coarsening patterns not observed for a mobile particle. The early time dynamics around initially still Janus colloids produces a force which is able to set the Janus colloid into motion. The propulsion due to this transient dynamics is in the direction opposite to that observed after the steady state is attained.

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link (url) DOI [BibTex]

2020


link (url) DOI [BibTex]


Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles
Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles

Singh, D., Domínguez, A., Choudhury, U., Kottapalli, S., Popescu, M., Dietrich, S., Fischer, P.

Nature Communications, 11(2210), May 2020 (article)

Abstract
Symmetry breaking and the emergence of self-organized patterns is the hallmark of com- plexity. Here, we demonstrate that a sessile drop, containing titania powder particles with negligible self-propulsion, exhibits a transition to collective motion leading to self-organized flow patterns. This phenomenology emerges through a novel mechanism involving the interplay between the chemical activity of the photocatalytic particles, which induces Mar- angoni stresses at the liquid–liquid interface, and the geometrical confinement provided by the drop. The response of the interface to the chemical activity of the particles is the source of a significantly amplified hydrodynamic flow within the drop, which moves the particles. Furthermore, in ensembles of such active drops long-ranged ordering of the flow patterns within the drops is observed. We show that the ordering is dictated by a chemical com- munication between drops, i.e., an alignment of the flow patterns is induced by the gradients of the chemicals emanating from the active particles, rather than by hydrodynamic interactions.

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link (url) DOI [BibTex]


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Axisymmetric spheroidal squirmers and self-diffusiophoretic particles

Pöhnl, R., Popescu, M. N., Uspal, W. E.

Journal of Physics: Condensed Matter, 32(16), IOP Publishing, Bristol, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Tracer diffusion on a crowded random Manhattan lattice

Mej\’\ia-Monasterio, C., Nechaev, S., Oshanin, G., Vasilyev, O.

New Journal of Physics, 22(3), IOP Publishing, Bristol, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Wetting transitions on soft substrates

Napiorkowski, M., Schimmele, L., Dietrich, S.

{EPL}, 129(1), EDP Science, Les-Ulis, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Blessing and Curse: How a Supercapacitor Large Capacitance Causes its Slow Charging

Lian, C., Janssen, M., Liu, H., van Roij, R.

Physical Review Letters, 124(7), American Physical Society, Woodbury, N.Y., 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Interplay of quenching temperature and drift in Brownian dynamics

Khalilian, H., Nejad, M. R., Moghaddam, A. G., Rohwer, C. M.

EPL, 128(6), EDP Science, Les-Ulis, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Fractal-seaweeds type functionalization of graphene

Amsharov, K., Sharapa, D. I., Vasilyev, O. A., Martin, O., Hauke, F., Görling, A., Soni, H., Hirsch, A.

Carbon, 158, pages: 435-448, Elsevier, Amsterdam, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Effective pair interaction of patchy particles in critical fluids

Farahmand Bafi, N., Nowakowski, P., Dietrich, S.

The Journal of Chemical Physics, 152(11), American Institute of Physics, Woodbury, N.Y., 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Cassie-Wenzel transition of a binary liquid mixture on a nanosculptured surface

Singh, S. L., Schimmele, L., Dietrich, S.

Physical Review E, 101(5), American Physical Society, Melville, NY, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Adopting the Boundary Homogenization Approximation from Chemical Kinetics to Motile Chemically Active Particles

Popescu, M. N., Uspal, W. E.

In Chemical Kinetics, pages: 517-540, World Scientific, New Jersey, NJ, 2020 (incollection)

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DOI [BibTex]

DOI [BibTex]


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Energy storage in steady states under cyclic local energy input

Zhang, Y., Holyst, R., Maciolek, A.

Physical Review E, 101(1), American Physical Society, Melville, NY, 2020 (article)

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Numerical simulations of self-diffusiophoretic colloids at fluid interfaces

Peter, T., Malgaretti, P., Rivas, N., Scagliarini, A., Harting, J., Dietrich, S.

Soft Matter, 16(14):3536-3547, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

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DOI [BibTex]

DOI [BibTex]

2011


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Collective dynamics of colloids at fluid interfaces

Bleibel, J., Dominguez, A., Oettel, M., Dietrich, S.

European Physical Journal E, 34(11), 2011 (article)

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2011


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Anomalous transport of a tracer on percolating clusters

Spanner, M., Höfling, F., Schröder-Turk, G. E., Mecke, K., Franosch, T.

Journal of Physics: Condensed Matter, 23(23), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Dynamics of colloids in confined geometries

Almenar, L., Rauscher, M.

Journal of Physics: Condensed Matter, 23(18), 2011 (article)

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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The structure and melting transition of two-dimensional colloidal alloys

Law, A. D., Horozov, T. S., Buzza, D. M. A.

Soft Matter, 7(19):8923-8931, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Second harmonic light scattering from spherical polyelectrolyte brushes

Schürer, B., Hoffmann, M., Wunderlich, S., Harnau, L., Peschel, U., Ballauff, M., Peukert, W.

Journal of Physical Chemistry C, 115, pages: 18302-18309, 2011 (article)

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DOI [BibTex]


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Simulation einer fast kritischen binären Flüssigkeit in einem Temperaturgradienten

Single, F.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Solvation forces in Ising films with long-range boundary fields: density-matrix renormalization-group study

Drzewinski, A., Maciolek, A., Barasinski, A.

Molecular Physics, 109(7-10):1133-1141, 2011 (article)

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DOI [BibTex]


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Pulling and pushing a cargo with a catalytically active carrier

Popescu, M. N., Tasinkevych, M., Dietrich, S.

Europhysics Letters, 95(2), 2011 (article)

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DOI [BibTex]


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Critical Casimir forces for Ising films with variable boundary fields

Vasilyev, O., Maciolek, A., Dietrich, S.

Physical Review E, 84(4), 2011 (article)

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Study of \pi\pi correlations at LHC and RHIC energies in pp collisions within the quark-gluon string model

Nilsson, M. S., Bravina, L. V., Zabrodin, E. E., Malinina, L. V., Bleibel, J.

Physical Review D, 84(5), 2011 (article)

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DOI [BibTex]


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Micro-rheology on (polymer-grafted) colloids using optical tweezers

Gutsche, C., Elmahdy, M. M., Kegler, K., Semenov, I., Stangner, T., Otto, O., Ueberschär, O., Keyser, U. F., Krüger, M., Rauscher, M., Weeber, R., Harting, J., Kim, Y. W., Lobaskin, V., Netz, R., Kremer, F.

Journal of Physics: Condensed Matter, 23(18), IOP Publishing, Bristol, 2011 (article)

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DOI [BibTex]


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Debye-Scherrer rings from block copolymer films with powder-like order

Busch, P., Rauscher, M., Moulin, J.-F., Müller-Buschbaum, P.

Journal of Applied Crystallography, 44(2):370-379, 2011 (article)

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DOI [BibTex]


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Effective interactions and equilibrium configurations of colloidal particles on a sessile droplet

Guzowski, J., Tasinkevych, M., Dietrich, S.

Soft Matter, 7(9):4189-4197, 2011 (article)

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DOI [BibTex]


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Capillary interactions in Pickering emulsions

Guzowski, J., Tasinkevych, M., Dietrich, S.

Physical Review E, 84(3), 2011 (article)

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DOI [BibTex]


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Critical Casimir forces steered by patterned substrates

Gambassi, A., Dietrich, S.

Soft Matter, 7(4):1247-1253, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Interaction strength between proteins and polyelectrolyte brushes: A small angle X-ray scattering study

Henzler, K., Haupt, B., Rosenfeldt, S., Harnau, L., Narayanan, T., Ballauff, M.

Physical Chemistry Chemical Physics, 13, pages: 17599-17605, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Annealing of single lamella nanoparticles of polyethylene

Rochette, C. N., Rosenfeldt, S., Henzler, K., Polzer, F., Ballauff, M., Tong, Q., Mecking, S., Drechsler, M., Narayanan, T., Harnau, L.

Macromolecules, 44(12):4845-4851, 2011 (article)

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DOI [BibTex]


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Struktur dichter ionischer Flüssigkeiten

Dannenmann, O.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Trapping colloids near chemical stripes via critical Casimir forces

Tröndle, M., Zvyagolskaya, O., Gambassi, A., Vogt, D., Harnau, L., Bechinger, C., Dietrich, S.

Molecular Physics, 109, pages: 1169-1185, 2011 (article)

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DOI [BibTex]


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Electrostatic interactions in critical solvents

Bier, M., Gambassi, A., Oettel, M., Dietrich, S.

Europhysics Letters, 95, 2011 (article)

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DOI [BibTex]


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Structural investigation of thin diblock copolymer films using time-of-flight grazing-incidence small-angle neutron scattering

Metwalli, E., Moulin, J.-F., Rauscher, M., Kaune, G., Ruderer, M. A., Van Bürck, U., Haese-Seiller, M., Kampmann, R., Müller-Buschbaum, P.

Journal of Applied Crystallography, 44(1):84-92, 2011 (article)

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DOI [BibTex]


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Complexation of beta-lactoglobulin fibrils and sulfated polysaccharides

Jones, O. G., Handschin, S., Adamcik, J., Harnau, L., Bolisetty, S., Mezzenga, R.

Biomacromolecules, 12, pages: 3056-3065, 2011 (article)

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DOI [BibTex]


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Parallelisierung Stokesscher Dynamik für Graphikprozessoren zur Simulation kolloidaler Suspensionen

Kopp, M.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Diffusion in Wandnähe

Müller, J.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Magnetization of multicomponent ferrofluids

Szalai, I., Dietrich, S.

Journal of Physics: Condensed Matter, 23(32), 2011 (article)

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DOI [BibTex]


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Space-resolved dynamics of a tracer in a disordered solid

Franosch, T., Spanner, M., Bauer, T., Schröder-Turk, G. E., Höfling, F.

Journal of Non-Crystalline Solids, 357(2):472-478, 2011 (article)

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Long-wavelength anomalies in the asymptotic behavior of mode-coupling theory

Schnyder, S. K., Höfling, F., Franosch, T., Voigtmann, T.

Journal of Physics: Condensed Matter, 23(23), 2011 (article)

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DOI [BibTex]

2003


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Effects of weak surface fields on the density profiles and adsorption of a confined fluid near bulk criticality

Maciolek, A., Evans, R., Wilding, N. B.

Journal of Chemical Physics, 119, pages: 8663-8675, 2003 (article)

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2003


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Orientational phase transition and the solvation force in a nematic liquid crystal confined between inhomogeneous subtrates

Kondrat, S., Poniewierski, A., Harnau, L.

European Physical Journal E, 10, pages: 163-170, 2003 (article)

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[BibTex]

[BibTex]


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Complex dewetting scenarios captured by thin-film models

Becker, J., Grün, G., Seeman, R., Mantz, H., Jacobs, K., Mecke, K. R., Blossey, R.

Nature Materials, 2, pages: 59-64, 2003 (article)

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[BibTex]


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Direct measurement of entropic forces induced by rigid rods

Helden, L., Roth, R., Koenderink, G. H., Leiderer, P., Bechinger, Clemens

Physical Review Letters, 90(4), 2003 (article)

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[BibTex]

[BibTex]


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On the reliability of initial conditions for dissipationless cosmological simulations

Knebe, A., Dominguez, A.

Publications of the Astronomical Society of Australia, 20, pages: 173-183, 2003 (article)

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[BibTex]

[BibTex]


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Wetting at curved substrates: Non-analytic behavior of interfacial properties

Evans, R., Roth, R., Bryk, P.

Europhysics Letters, 62(6):815-821, 2003 (article)

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[BibTex]

[BibTex]


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Transverse fluctuations in the driven lattice gas

Caracciolo, S., Gambassi, A., Gubinelli, M., Pelissetto, A.

Journal of Physics A, 36, pages: L315-L320, 2003 (article)

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[BibTex]

[BibTex]


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Depletion potentials in colloidal mixtures of spheres and rods

Roth, R.

Journal of Physics: Condensed Matter, 15, pages: S277-S282, 2003 (article)

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[BibTex]

[BibTex]


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Universality of the thermodynamic Casimir effect

Dantchev, D. M., Krech, M., Dietrich, S.

Physical Review E, 67, 2003 (article)

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[BibTex]

[BibTex]