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2011


Quantum-Cascade Laser-Based Vibrational Circular Dichroism
Quantum-Cascade Laser-Based Vibrational Circular Dichroism

Luedeke, S., Pfeifer, M., Fischer, P.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 133(15):5704-5707, 2011 (article)

Abstract
Vibrational circular dichroism (VCD) spectra were recorded with a tunable external-cavity quantum-cascade laser (QCL). In comparison with standard thermal light sources in the IR, QCLs provide orders of magnitude more power and are therefore promising for VCD studies in strongly absorbing solvents. The brightness of this novel light source is demonstrated with VCD and IR absorption measurements of a number of compounds, including proline in water.

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DOI [BibTex]

2011


DOI [BibTex]


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Collective dynamics of colloids at fluid interfaces

Bleibel, J., Dominguez, A., Oettel, M., Dietrich, S.

European Physical Journal E, 34(11), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Anomalous transport of a tracer on percolating clusters

Spanner, M., Höfling, F., Schröder-Turk, G. E., Mecke, K., Franosch, T.

Journal of Physics: Condensed Matter, 23(23), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Dynamics of colloids in confined geometries

Almenar, L., Rauscher, M.

Journal of Physics: Condensed Matter, 23(18), 2011 (article)

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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The structure and melting transition of two-dimensional colloidal alloys

Law, A. D., Horozov, T. S., Buzza, D. M. A.

Soft Matter, 7(19):8923-8931, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Second harmonic light scattering from spherical polyelectrolyte brushes

Schürer, B., Hoffmann, M., Wunderlich, S., Harnau, L., Peschel, U., Ballauff, M., Peukert, W.

Journal of Physical Chemistry C, 115, pages: 18302-18309, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Simulation einer fast kritischen binären Flüssigkeit in einem Temperaturgradienten

Single, F.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


Actively coupled cavity ringdown spectroscopy with low-power broadband sources
Actively coupled cavity ringdown spectroscopy with low-power broadband sources

Petermann, C., Fischer, P.

OPTICS EXPRESS, 19(11):10164-10173, 2011 (article)

Abstract
We demonstrate a coupling scheme for cavity enhanced absorption spectroscopy that makes use of an intracavity acousto-optical modulator to actively switch light into (and out of) a resonator. This allows cavity ringdown spectroscopy (CRDS) to be implemented with broadband nonlaser light sources with spectral power densities of less than 30 mu W/nm. Although the acousto-optical element reduces the ultimate detection limit by introducing additional losses, it permits absorptivities to be measured with a high dynamic range, especially in lossy environments. Absorption measurements for the forbidden transition of gaseous oxygen in air at similar to 760nm are presented using a low-coherence cw-superluminescent diode. The same setup was electronically configured to cover absorption losses from 1.8 x 10(-8)cm(-1) to 7.5\% per roundtrip. This could be of interest in process analytical applications. (C) 2011 Optical Society of America

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DOI [BibTex]

DOI [BibTex]


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Solvation forces in Ising films with long-range boundary fields: density-matrix renormalization-group study

Drzewinski, A., Maciolek, A., Barasinski, A.

Molecular Physics, 109(7-10):1133-1141, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Pulling and pushing a cargo with a catalytically active carrier

Popescu, M. N., Tasinkevych, M., Dietrich, S.

Europhysics Letters, 95(2), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Critical Casimir forces for Ising films with variable boundary fields

Vasilyev, O., Maciolek, A., Dietrich, S.

Physical Review E, 84(4), 2011 (article)

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DOI [BibTex]


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Study of \pi\pi correlations at LHC and RHIC energies in pp collisions within the quark-gluon string model

Nilsson, M. S., Bravina, L. V., Zabrodin, E. E., Malinina, L. V., Bleibel, J.

Physical Review D, 84(5), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Micro-rheology on (polymer-grafted) colloids using optical tweezers

Gutsche, C., Elmahdy, M. M., Kegler, K., Semenov, I., Stangner, T., Otto, O., Ueberschär, O., Keyser, U. F., Krüger, M., Rauscher, M., Weeber, R., Harting, J., Kim, Y. W., Lobaskin, V., Netz, R., Kremer, F.

Journal of Physics: Condensed Matter, 23(18), IOP Publishing, Bristol, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Debye-Scherrer rings from block copolymer films with powder-like order

Busch, P., Rauscher, M., Moulin, J.-F., Müller-Buschbaum, P.

Journal of Applied Crystallography, 44(2):370-379, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


Magnetically actuated propulsion at low Reynolds numbers: towards nanoscale control
Magnetically actuated propulsion at low Reynolds numbers: towards nanoscale control

Fischer, P., Ghosh, A.

NANOSCALE, 3(2):557-563, 2011 (article)

Abstract
Significant progress has been made in the fabrication of micron and sub-micron structures whose motion can be controlled in liquids under ambient conditions. The aim of many of these engineering endeavors is to be able to build and propel an artificial micro-structure that rivals the versatility of biological swimmers of similar size, e. g. motile bacterial cells. Applications for such artificial ``micro-bots'' are envisioned to range from microrheology to targeted drug delivery and microsurgery, and require full motion-control under ambient conditions. In this Mini-Review we discuss the construction, actuation, and operation of several devices that have recently been reported, especially systems that can be controlled by and propelled with homogenous magnetic fields. We describe the fabrication and associated experimental challenges and discuss potential applications.

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Video - Nanospropellers DOI [BibTex]


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Effective interactions and equilibrium configurations of colloidal particles on a sessile droplet

Guzowski, J., Tasinkevych, M., Dietrich, S.

Soft Matter, 7(9):4189-4197, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Capillary interactions in Pickering emulsions

Guzowski, J., Tasinkevych, M., Dietrich, S.

Physical Review E, 84(3), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Critical Casimir forces steered by patterned substrates

Gambassi, A., Dietrich, S.

Soft Matter, 7(4):1247-1253, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Interaction strength between proteins and polyelectrolyte brushes: A small angle X-ray scattering study

Henzler, K., Haupt, B., Rosenfeldt, S., Harnau, L., Narayanan, T., Ballauff, M.

Physical Chemistry Chemical Physics, 13, pages: 17599-17605, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Annealing of single lamella nanoparticles of polyethylene

Rochette, C. N., Rosenfeldt, S., Henzler, K., Polzer, F., Ballauff, M., Tong, Q., Mecking, S., Drechsler, M., Narayanan, T., Harnau, L.

Macromolecules, 44(12):4845-4851, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Struktur dichter ionischer Flüssigkeiten

Dannenmann, O.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Trapping colloids near chemical stripes via critical Casimir forces

Tröndle, M., Zvyagolskaya, O., Gambassi, A., Vogt, D., Harnau, L., Bechinger, C., Dietrich, S.

Molecular Physics, 109, pages: 1169-1185, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Electrostatic interactions in critical solvents

Bier, M., Gambassi, A., Oettel, M., Dietrich, S.

Europhysics Letters, 95, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Structural investigation of thin diblock copolymer films using time-of-flight grazing-incidence small-angle neutron scattering

Metwalli, E., Moulin, J.-F., Rauscher, M., Kaune, G., Ruderer, M. A., Van Bürck, U., Haese-Seiller, M., Kampmann, R., Müller-Buschbaum, P.

Journal of Applied Crystallography, 44(1):84-92, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Complexation of beta-lactoglobulin fibrils and sulfated polysaccharides

Jones, O. G., Handschin, S., Adamcik, J., Harnau, L., Bolisetty, S., Mezzenga, R.

Biomacromolecules, 12, pages: 3056-3065, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Parallelisierung Stokesscher Dynamik für Graphikprozessoren zur Simulation kolloidaler Suspensionen

Kopp, M.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


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Diffusion in Wandnähe

Müller, J.

Universität Stuttgart, Stuttgart, 2011 (mastersthesis)

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[BibTex]

[BibTex]


Weak value amplified optical activity measurements
Weak value amplified optical activity measurements

Pfeifer, M., Fischer, P.

Opt. Express, 19(17):16508-16517, OSA, 2011 (article)

Abstract
We present a new form of optical activity measurement based on a modified weak value amplification scheme. It has recently been shown experimentally that the left- and right-circular polarization components refract with slightly different angles of refraction at a chiral interface causing a linearly polarized light beam to split into two. By introducing a polarization modulation that does not give rise to a change in the optical rotation it is possible to differentiate between the two circular polarization components even after post-selection with a linear polarizer. We show that such a modified weak value amplification measurement permits the sign of the splitting and thus the handedness of the optically active medium to be determined. Angular beam separations of Δθ ∼ 1 nanoradian, which corresponds to a circular birefringence of Δn ∼ 1 × 10−9, could be measured with a relative error of less than 1%.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Magnetization of multicomponent ferrofluids

Szalai, I., Dietrich, S.

Journal of Physics: Condensed Matter, 23(32), 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Space-resolved dynamics of a tracer in a disordered solid

Franosch, T., Spanner, M., Bauer, T., Schröder-Turk, G. E., Höfling, F.

Journal of Non-Crystalline Solids, 357(2):472-478, 2011 (article)

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DOI [BibTex]

DOI [BibTex]


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Long-wavelength anomalies in the asymptotic behavior of mode-coupling theory

Schnyder, S. K., Höfling, F., Franosch, T., Voigtmann, T.

Journal of Physics: Condensed Matter, 23(23), 2011 (article)

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DOI [BibTex]

DOI [BibTex]

2003


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Effects of weak surface fields on the density profiles and adsorption of a confined fluid near bulk criticality

Maciolek, A., Evans, R., Wilding, N. B.

Journal of Chemical Physics, 119, pages: 8663-8675, 2003 (article)

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[BibTex]

2003


[BibTex]


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Orientational phase transition and the solvation force in a nematic liquid crystal confined between inhomogeneous subtrates

Kondrat, S., Poniewierski, A., Harnau, L.

European Physical Journal E, 10, pages: 163-170, 2003 (article)

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[BibTex]

[BibTex]


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Complex dewetting scenarios captured by thin-film models

Becker, J., Grün, G., Seeman, R., Mantz, H., Jacobs, K., Mecke, K. R., Blossey, R.

Nature Materials, 2, pages: 59-64, 2003 (article)

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[BibTex]

[BibTex]


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Direct measurement of entropic forces induced by rigid rods

Helden, L., Roth, R., Koenderink, G. H., Leiderer, P., Bechinger, Clemens

Physical Review Letters, 90(4), 2003 (article)

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[BibTex]

[BibTex]


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On the reliability of initial conditions for dissipationless cosmological simulations

Knebe, A., Dominguez, A.

Publications of the Astronomical Society of Australia, 20, pages: 173-183, 2003 (article)

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[BibTex]

[BibTex]


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Wetting at curved substrates: Non-analytic behavior of interfacial properties

Evans, R., Roth, R., Bryk, P.

Europhysics Letters, 62(6):815-821, 2003 (article)

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[BibTex]

[BibTex]


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Transverse fluctuations in the driven lattice gas

Caracciolo, S., Gambassi, A., Gubinelli, M., Pelissetto, A.

Journal of Physics A, 36, pages: L315-L320, 2003 (article)

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[BibTex]

[BibTex]


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Depletion potentials in colloidal mixtures of spheres and rods

Roth, R.

Journal of Physics: Condensed Matter, 15, pages: S277-S282, 2003 (article)

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[BibTex]

[BibTex]


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Universality of the thermodynamic Casimir effect

Dantchev, D. M., Krech, M., Dietrich, S.

Physical Review E, 67, 2003 (article)

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[BibTex]

[BibTex]


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Singularities and spatial fluctuations in submonolayer epitaxy - Reply

Amar, J. G., Popescu, M. N., Family, F.

Physical Review Letters, 90(18), 2003 (article)

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[BibTex]

[BibTex]


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Critical Casimir forces in colloidal suspensions

Schlesener, F., Hanke, A., Dietrich, S.

Journal of Statistical Physics, 110, pages: 981-1013, 2003 (article)

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[BibTex]

[BibTex]


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Coexisting Phases in Binary Platelet Mixtures

Bier, M.

Universität Stuttgart, Stuttgart, 2003 (mastersthesis)

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[BibTex]

[BibTex]


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Reconstructing complex materials via effective grain shapes

Arns, C. H., Knackstedt, M. A., Mecke, K. R.

Physical Review Letters, 91, 2003 (article)

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[BibTex]

[BibTex]


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Capillary forces between structured substrates

De Souza, E. J.

Universität Stuttgart, Stuttgart, 2003 (mastersthesis)

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[BibTex]

[BibTex]


New electro-optic effect: Sum-frequency generation from optically active liquids in the presence of a dc electric field
New electro-optic effect: Sum-frequency generation from optically active liquids in the presence of a dc electric field

Fischer, P., Buckingham, A., Beckwitt, K., Wiersma, D., Wise, F.

PHYSICAL REVIEW LETTERS, 91(17), 2003 (article)

Abstract
We report the observation of sum-frequency signals that depend linearly on an applied electrostatic field and that change sign with the handedness of an optically active solute. This recently predicted chiral electro-optic effect exists in the electric-dipole approximation. The static electric field gives rise to an electric-field-induced sum-frequency signal (an achiral third-order process) that interferes with the chirality-specific sum-frequency at second order. The cross-terms linear in the electrostatic field constitute the effect and may be used to determine the absolute sign of second- and third-order nonlinear-optical susceptibilities in isotropic media.

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DOI [BibTex]

DOI [BibTex]


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Depletion potentials near geometrically structured substrates

Bryk, P., Roth, R., Schoen, M., Dietrich, S.

Europhysics Letters, 63(2):233-239, 2003 (article)

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[BibTex]

[BibTex]


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Diffusion in polymer-derived Si-(B-)C-N ceramics, particularly amorphous Si29B9C41N21

Voss, T., Strohm, A., Frank, W.

Zeitschrift f\"ur Metallkunde, 94(4):419-423, 2003 (article)

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[BibTex]

[BibTex]