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2020


Transient coarsening and the motility of optically heated Janus colloids in a binary liquid mixture
Transient coarsening and the motility of optically heated Janus colloids in a binary liquid mixture

Gomez-Solano, J., Roy, S., Araki, T., Dietrich, S., Maciolek, A.

Soft Matter, 16, pages: 8359-8371, Royal Society of Chemistry, August 2020 (article)

Abstract
A gold-capped Janus particle suspended in a near-critical binary liquid mixture can self-propel under illumination. We have immobilized such a particle in a narrow channel and carried out a combined experimental and theoretical study of the non-equilibrium dynamics of a binary solvent around it – lasting from the very moment of switching illumination on until the steady state is reached. In the theoretical study we use both a purely diffusive and a hydrodynamic model, which we solve numerically. Our results demonstrate a remarkable complexity of the time evolution of the concentration field around the colloid. This evolution is governed by the combined effects of the temperature gradient and the wettability, and crucially depends on whether the colloid is free to move or is trapped. For the trapped colloid, all approaches indicate that the early time dynamics is purely diffusive and characterized by composition layers travelling with constant speed from the surface of the colloid into the bulk of the solvent. Subsequently, hydrodynamic effects set in. Anomalously large nonequilibrium fluctuations, which result from the temperature gradient and the vicinity of the critical point of the binary liquid mixture, give rise to strong concentration fluctuations in the solvent and to permanently changing coarsening patterns not observed for a mobile particle. The early time dynamics around initially still Janus colloids produces a force which is able to set the Janus colloid into motion. The propulsion due to this transient dynamics is in the direction opposite to that observed after the steady state is attained.

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link (url) DOI [BibTex]

2020


link (url) DOI [BibTex]


Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles
Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles

Singh, D., Domínguez, A., Choudhury, U., Kottapalli, S., Popescu, M., Dietrich, S., Fischer, P.

Nature Communications, 11(2210), May 2020 (article)

Abstract
Symmetry breaking and the emergence of self-organized patterns is the hallmark of com- plexity. Here, we demonstrate that a sessile drop, containing titania powder particles with negligible self-propulsion, exhibits a transition to collective motion leading to self-organized flow patterns. This phenomenology emerges through a novel mechanism involving the interplay between the chemical activity of the photocatalytic particles, which induces Mar- angoni stresses at the liquid–liquid interface, and the geometrical confinement provided by the drop. The response of the interface to the chemical activity of the particles is the source of a significantly amplified hydrodynamic flow within the drop, which moves the particles. Furthermore, in ensembles of such active drops long-ranged ordering of the flow patterns within the drops is observed. We show that the ordering is dictated by a chemical com- munication between drops, i.e., an alignment of the flow patterns is induced by the gradients of the chemicals emanating from the active particles, rather than by hydrodynamic interactions.

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link (url) DOI [BibTex]


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Axisymmetric spheroidal squirmers and self-diffusiophoretic particles

Pöhnl, R., Popescu, M. N., Uspal, W. E.

Journal of Physics: Condensed Matter, 32(16), IOP Publishing, Bristol, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Tracer diffusion on a crowded random Manhattan lattice

Mej\’\ia-Monasterio, C., Nechaev, S., Oshanin, G., Vasilyev, O.

New Journal of Physics, 22(3), IOP Publishing, Bristol, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Wetting transitions on soft substrates

Napiorkowski, M., Schimmele, L., Dietrich, S.

{EPL}, 129(1), EDP Science, Les-Ulis, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Blessing and Curse: How a Supercapacitor Large Capacitance Causes its Slow Charging

Lian, C., Janssen, M., Liu, H., van Roij, R.

Physical Review Letters, 124(7), American Physical Society, Woodbury, N.Y., 2020 (article)

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DOI [BibTex]

DOI [BibTex]


Wearable and Stretchable Strain Sensors: Materials, Sensing Mechanisms, and Applications
Wearable and Stretchable Strain Sensors: Materials, Sensing Mechanisms, and Applications

Souri, H., Banerjee, H., Jusufi, A., Radacsi, N., Stokes, A. A., Park, I., Sitti, M., Amjadi, M.

Advanced Intelligent Systems, 2020 (article)

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Interplay of quenching temperature and drift in Brownian dynamics

Khalilian, H., Nejad, M. R., Moghaddam, A. G., Rohwer, C. M.

EPL, 128(6), EDP Science, Les-Ulis, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Fractal-seaweeds type functionalization of graphene

Amsharov, K., Sharapa, D. I., Vasilyev, O. A., Martin, O., Hauke, F., Görling, A., Soni, H., Hirsch, A.

Carbon, 158, pages: 435-448, Elsevier, Amsterdam, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Effective pair interaction of patchy particles in critical fluids

Farahmand Bafi, N., Nowakowski, P., Dietrich, S.

The Journal of Chemical Physics, 152(11), American Institute of Physics, Woodbury, N.Y., 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Cassie-Wenzel transition of a binary liquid mixture on a nanosculptured surface

Singh, S. L., Schimmele, L., Dietrich, S.

Physical Review E, 101(5), American Physical Society, Melville, NY, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Fish-like aquatic propulsion studied using a pneumatically-actuated soft-robotic model

Wolf, Z., Jusufi, A., Vogt, D. M., Lauder, G. V.

Bioinspiration & Biomimetics, 15(4):046008, Inst. of Physics, London, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Adopting the Boundary Homogenization Approximation from Chemical Kinetics to Motile Chemically Active Particles

Popescu, M. N., Uspal, W. E.

In Chemical Kinetics, pages: 517-540, World Scientific, New Jersey, NJ, 2020 (incollection)

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DOI [BibTex]

DOI [BibTex]


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Energy storage in steady states under cyclic local energy input

Zhang, Y., Holyst, R., Maciolek, A.

Physical Review E, 101(1), American Physical Society, Melville, NY, 2020 (article)

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DOI [BibTex]

DOI [BibTex]


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Numerical simulations of self-diffusiophoretic colloids at fluid interfaces

Peter, T., Malgaretti, P., Rivas, N., Scagliarini, A., Harting, J., Dietrich, S.

Soft Matter, 16(14):3536-3547, Royal Society of Chemistry, Cambridge, UK, 2020 (article)

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DOI [BibTex]

DOI [BibTex]

2019


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Aging phenomena during phase separation in fluids: decay of autocorrelation for vapor-liquid transitions

Roy, S., Bera, A., Majumder, S., Das, S. K.

Soft Matter, 15(23):4743-4750, Royal Society of Chemistry, Cambridge, UK, May 2019 (article)

Abstract
We performed molecular dynamics simulations to study relaxation phenomena during vapor–liquid transitions in a single component Lennard-Jones system. Results from two different overall densities are presented: one in the neighborhood of the vapor branch of the coexistence curve and the other being close to the critical density. The nonequilibrium morphologies, growth mechanisms and growth laws in the two cases are vastly different. In the low density case growth occurs via diffusive coalescence of droplets in a disconnected morphology. On the other hand, the elongated structure in the higher density case grows via advective transport of particles inside the tube-like liquid domains. The objective in this work has been to identify how the decay of the order-parameter autocorrelation, an important quantity to understand aging dynamics, differs in the two cases. In the case of the disconnected morphology, we observe a very robust power-law decay, as a function of the ratio of the characteristic lengths at the observation time and at the age of the system, whereas the results for the percolating structure appear rather complex. To quantify the decay in the latter case, unlike the standard method followed in a previous study, here we have performed a finite-size scaling analysis. The outcome of this analysis shows the presence of a strong preasymptotic correction, while revealing that in this case also, albeit in the asymptotic limit, the decay follows a power-law. Even though the corresponding exponents in the two cases differ drastically, this study, combined with a few recent ones, suggests that power-law behavior of this correlation function is rather universal in coarsening dynamics.

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link (url) DOI [BibTex]

2019


link (url) DOI [BibTex]


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Response of active Brownian particles to shear flow

Asheichyk, K., Solon, A., Rohwer, C. M., Krüger, M.

The Journal of Chemical Physics, 150(14), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Vortex Mass in the Three-Dimensional O(2) Scalar Theory

Delfino, G., Selke, W., Squarcini, A.

Physical Review Letters, 122(5), American Physical Society, Woodbury, N.Y., 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Ferromagnetic colloids in liquid crystal solvents

Zarubin, G.

Universität Stuttgart, Stuttgart, 2019 (phdthesis)

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Fluctuating interface with a pinning potential

Pranjić, Daniel

Universität Stuttgart, Stuttgart, 2019 (mastersthesis)

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[BibTex]

[BibTex]


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Dynamics near planar walls for various model self-phoretic particles

Bayati, P., Popescu, M. N., Uspal, W. E., Dietrich, S., Najafi, A.

Soft Matter, 15(28):5644-5672, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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DOI [BibTex]


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Glucose Oxidase Micropumps: Multi-Faceted Effects of Chemical Activity on Tracer Particles Near the Solid-Liquid Interface

Munteanu, R. E., Popescu, M. N., Gáspár, S.

Condensed Matter, 4(3), MDPI, Basel, 2019 (article)

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Criticality senses topology

Vasilyev, O. A., Maciolek, A., Dietrich, S.

EPL, 128(2), EDP Science, Les-Ulis, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Soft Sensors for Curvature Estimation under Water in a Soft Robotic Fish

Wright, Brian, Vogt, Daniel M., Wood, Robert J., Jusufi, Ardian

In 2019 2nd IEEE International Conference on Soft Robotics (RoboSoft 2019), pages: 367-371, IEEE, Piscataway, NJ, 2nd IEEE International Conference on Soft Robotics (RoboSoft 2019), 2019 (inproceedings)

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DOI [BibTex]


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Drag Force for Asymmetrically Grafted Colloids in Polymer Solutions

Werner, M., Malgaretti, P., Maciolek, A.

Frontiers in Physics, 7, Frontiers Media, Lausanne, 2019 (article)

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DOI [BibTex]


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Feeling Your Neighbors across the Walls: How Interpore Ionic Interactions Affect Capacitive Energy Storage

Kondrat, S., Vasilyev, O., Kornyshev, A. A.

The Journal of Physical Chemistry Letters, 10(16):4523-4527, American Chemical Society, Washington, DC, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Active Janus colloids at chemically structured surfaces

Uspal, W. E., Popescu, M. N., Dietrich, S., Tasinkevych, M.

The Journal of Chemical Physics, 150(20), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Illumination-induced motion of a Janus nanoparticle in binary solvents

Araki, T., Maciolek, A.

Soft Matter, 15(26):5243-5254, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Transient response of an electrolyte to a thermal quench

Janssen, M., Bier, M.

Physical Review E, 99(4), American Physical Society, Melville, NY, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Controlling pattern formation in the confined Schnakenberg model

Beyer, David Bernhard

Universität Stuttgart, Stuttgart, 2019 (mastersthesis)

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[BibTex]

[BibTex]


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Flux and storage of energy in nonequilibrium stationary states

Holyst, R., Maciolek, A., Zhang, Y., Litniewski, M., Knycha\la, P., Kasprzak, M., Banaszak, M.

Physical Review E, 99(4), American Physical Society, Melville, NY, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Correlations and forces in sheared fluids with or without quenching

Rohwer, C. M., Maciolek, A., Dietrich, S., Krüger, M.

New Journal of Physics, 21, IOP Publishing, Bristol, 2019 (article)

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Ensemble dependence of critical Casimir forces in films with Dirichlet boundary conditions

Rohwer, C. M., Squarcini, A., Vasilyev, O., Dietrich, S., Gross, M.

Physical Review E, 99(6), American Physical Society, Melville, NY, 2019 (article)

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DOI [BibTex]


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Controlling the dynamics of colloidal particles by critical Casimir forces

Magazzù, A., Callegari, A., Staforelli, J. P., Gambassi, A., Dietrich, S., Volpe, G.

Soft Matter, 15(10):2152-2162, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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DOI [BibTex]


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Charge regulation radically modifies electrostatics in membrane stacks

Majee, A., Bier, M., Blossey, R., Podgornik, R.

Physical Review E, 100(5), American Physical Society, Melville, NY, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Co-Contraction facilitates Body Stiffness Modulation during Swimming with Sensory Feedback in a Soft Biorobotic Physical Model

Jusufi, A., Vogt, D., Wood, R. J.

Integrative and Comparative Biology, 59(Supplement 1):E116-E116, Society of Integrative and Comparative Biology, McLean, VA, 2019 (article)

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DOI [BibTex]


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Comment on "Which interactions dominate in active colloids?" [J. Chem. Phys. 150, 061102 (2019)]

Popescu, M. N., Dominguez, A., Uspal, W. E., Tasinkevych, M., Dietrich, S.

The Journal of Chemical Physics, 151(6), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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DOI [BibTex]


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Current-mediated synchronization of a pair of beating non-identical flagella

Dotsenko, V., Maciolek, A., Oshanin, G., Vasilyev, O., Dietrich, S.

New Journal of Physics, 21, IOP Publishing, Bristol, 2019 (article)

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DOI [BibTex]


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Driving an electrolyte through a corrugated nanopore

Malgaretti, P., Janssen, M., Pagonabarraga, I., Rubi, J. M.

The Journal of Chemical Physics, 151(8), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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DOI [BibTex]


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Interfaces in fluids of ionic liquid crystals

Bartsch, H.

Universität Stuttgart, Stuttgart, 2019 (phdthesis)

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Spectral Content of a Single Non-Brownian Trajectory

Krapf, D., Lukat, N., Marinari, E., Metzler, R., Oshanin, G., Selhuber-Unkel, C., Squarcini, A., Stadler, L., Weiss, M., Xu, X.

Physical Review X, 9(1), American Physical Society, New York, NY, 2019 (article)

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DOI [BibTex]


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Special issue on transport in narrow channels
Journal of Physics: Condensed Matter, 31, IOP Publishing, Bristol, 2019 (misc)

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Curvature affects electrolyte relaxation: Studies of spherical and cylindrical electrodes

Janssen, M.

Physical Review E, 100(4), American Physical Society, Melville, NY, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Dynamics of the critical Casimir force for a conserved order parameter after a critical quench

Gross, M., Rohwer, C. M., Dietrich, S.

Physical Review E, 100(1), American Physical Society, Melville, NY, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Interface structures in ionic liquid crystals

Bartsch, H., Bier, M., Dietrich, S.

Soft Matter, 15(20):4109-4126, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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DOI [BibTex]

DOI [BibTex]


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Interfacial premelting of ice in nano composite materials

Li, H., Bier, M., Mars, J., Weiss, H., Dippel, A., Gutowski, O., Honkimäki, V., Mezger, M.

Physical Chemistry Chemical Physics, 21(7):3734-3741, Royal Society of Chemistry, Cambridge, England, 2019 (article)

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Connections Matter: On the Importance of Pore Percolation for Nanoporous Supercapacitors

Vasilyev, O., Kornyshev, A. A., Kondrat, S.

ACS Applied Energy Materials, 2(8):5386-5390, American Chemical Society, Washington, DC, 2019 (article)

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DOI [BibTex]


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Theory of light-activated catalytic Janus particles

Uspal, W. E.

The Journal of Chemical Physics, 150(11), American Institute of Physics, Woodbury, N.Y., 2019 (article)

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DOI [BibTex]


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Recovering superhydrophobicity in nanoscale and macroscale surface textures

Giacomello, A., Schimmele, L., Dietrich, S., Tasinkevych, M.

Soft Matter, 15(37):7462-7471, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

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DOI [BibTex]